Author: Schubert, S.G.
Paper Title Page
WEPWA032 CsK2Sb Growth Studies: Towards High Quantum Efficiency and Smooth Surfaces 2566
 
  • S.G. Schubert, M. Gaowei, J. Sinsheimer, J. Smedley
    BNL, Upton, Long Island, New York, USA
  • Z. Ding, E.M. Muller
    SBU, Stony Brook, New York, USA
  • J. Kühn
    HZB, Berlin, Germany
  • H.A. Padmore, J.J. Wong
    LBNL, Berkeley, California, USA
  • J. Xie
    ANL, Argonne, Illinois, USA
 
  Funding: This work was supported by the US DOE, under Contracts DE-AC02-05CH11231, DE-AC02-98CH10886, KC0407-ALSJNT-I0013, DE-FG02-12ER41837 and the German BMBF, Helmholtz-Association and Land Berlin.
The properties of CsK2Sb, make this material an ideal candidate as photocathode for electron injector use. Producing photocathodes with quantum efficiencies with 7% and greater at 532 nm poses no challenge, nevertheless the traditional growth mechanisms, which are based on a sequential deposition of Antimony, Potassium and Cesium at a temperature gradient yield a rough surface with a rms roughness in the range of 25 nm. Surface roughness’s in this region impacts the emittance. At an accelerating field of 3 MV/m an rms surface roughness of 25 nm is the dominant effect on emittance and will limit injector performance. Studies are performed to optimize roughness. Various growth procedures are exploited and the surface roughness compared.
 
DOI • reference for this paper ※ https://doi.org/10.18429/JACoW-IPAC2015-WEPWA032  
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TUPHA003 Sputter Growth of Alkali Antimonide Photocathodes: An in Operando Materials Analysis 1965
 
  • J. Smedley, K. Attenkofer, M. Gaowei, J. Sinsheimer, J. Walsh
    BNL, Upton, Long Island, New York, USA
  • H. Bhandari
    Radiation Monitoring Devices, Watertown, USA
  • Z. Ding, E.M. Muller
    SBU, Stony Brook, New York, USA
  • H.J. Frisch
    Enrico Fermi Institute, University of Chicago, Chicago, Illinois, USA
  • H.A. Padmore, S.G. Schubert, J.J. Wong
    LBNL, Berkeley, California, USA
 
  Funding: Work supported by U.S. DoE, under KC0407-ALSJNT-I0013 and SBIR grant # DE-SC0009540. NSLS was supported by DOE DE-AC02-98CH10886, CHESS is supported by NSF & NIH/NIGMS via NSF DMR-1332208
Alkali antimonide photocathodes are a strong contender for the cathode of choice for next-generation photon sources such as LCLS II or the XFEL. These materials have already found extensive use in photodetectors and image intensifiers. However, only recently have modern synchrotron techniques enabled a systematic study of the formation chemistry of these materials. Such analysis has led to the understanding that these materials are inherently rough when grown through traditional sequential deposition; this roughness has a detrimental impact on the intrinsic emittance of the emitted beam. Sputter deposition may provide a path to achieving a far smoother photocathode, while maintaining adequate quantum efficiency. We report on the creation and vacuum transport of a K2CsSb sputter target, and its use to create an ultra-smooth (sub nm roughness) cathode with a 2% quantum efficiency at 532 nm.
 
DOI • reference for this paper ※ https://doi.org/10.18429/JACoW-IPAC2015-TUPHA003  
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